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Efficient dechlorination of 2,4-dichlorophenol in an aqueous media with a mild pH using a Pd/TiO

Jiangkun DU,Jianguo BAO,Wei HU

Frontiers of Environmental Science & Engineering 2015, Volume 9, Issue 5,   Pages 919-928 doi: 10.1007/s11783-015-0794-x

Abstract: In this study, palladium-loaded titania nanotubes was fabricated on a titanium plate (Pd/TiO NTs/Ti)for efficient electrodechlorination of 2,4-chlorophenol with a mild pH condition.The nature of Pd/TiO NTs/Ti electrodes was characterized by field-emission scanning electron microscopeon titania nanotubes arrays on the Pd/TiO NTs/Ti surface.Furthermore, the intermediates analysis showed that the Pd/TiO NTs/Ti electrode could completely remove

Keywords： Pd/TiO<sub>2sub>NTs/Ti cathode     chlorophenols     electrocatalytic dechlorination     wastewater treatment    

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Effective regeneration of thermally deactivated commercial V-W-Ti catalysts

Xuesong SHANG, Jianrong LI, Xiaowei YU, Jinsheng CHEN, Chi HE

Frontiers of Chemical Science and Engineering 2012, Volume 6, Issue 1,   Pages 38-46 doi: 10.1007/s11705-011-1167-z

Abstract: An effective method for the regeneration of thermally deactivated commercial monolith SCR catalysts was investigated. Two types of regenerated solutions, namely NH Cl (1 mol/L) and dilute H SO (0.5 mol/L), were employed to treat the used catalyst. The effects of temperature and the regeneration process on the structural and textural properties of the catalysts were determined by X-ray diffraction, scanning electron microscopy, N adsorption/desorption, elemental analysis and Fourier transform infrared spectroscopy. The results suggest that the anatase phase of the used catalyst is maintained after exposure to high temperatures. Some of the catalytic activity was restored after regeneration. The catalyst regenerated by aqueous NH Cl had a higher activity than that of the catalyst treated by dilute H SO . The main reason is that the NH generated from the decomposition of NH Cl at high temperatures can be adsorbed onto the catalyst which promotes the reaction. The aggregated V O were partially re-dispersed during the regeneration process, and the intrinsic oxidation of ammonia with high concentrations of O is a factor that suppresses the catalytic activity.

Keywords： V<sub>2sub>O<sub>5sub>-WO<sub>3sub>/TiO<sub>2sub> catalysts     thermal deactivation     regeneration     NH<sub>4sub>Cl     dilute H<sub>2sub>SO<sub>4sub> solution    

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Interfacial charge transfer and photocatalytic activity in a reverse designed BiO/TiO core-shell

Frontiers in Energy 2021, Volume 15, Issue 3,   Pages 732-743 doi: 10.1007/s11708-021-0772-x

Abstract: photocatalytic properties of core-shell heterojunctions photocatalysts with reversible configuration of TiO<sub>2sub> and Bi<sub>2sub>O<sub>3sub> layers were studied.The results show the formation of homogenous TiO<sub>2sub> anatase and Bi<sub>2sub>O<sub>3sub>In optimal core-shell design, Bi<sub>2sub>O<sub>3sub> collects holes from TiO<sub>2sub>, leavingelectrons free to react and increase by 5 times the photocatalytic efficiency toward H<sub>2sub> generation

Keywords： photocatalysis     core-shell     heterojunction     H<sub>2sub>     TiO<sub>2sub>     Bi<sub>2sub>O<sub>3sub    

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Synthesis, physicochemical characterizations and catalytic performance of Pd/carbon-zeolite and Pd/carbon-CeO

Zeinab JAMALZADEH, Mohammad HAGHIGHI, Nazli ASGARI

Frontiers of Environmental Science & Engineering 2013, Volume 7, Issue 3,   Pages 365-381 doi: 10.1007/s11783-013-0520-5

Abstract: In this work, xylene removal from waste gas streams was investigated via catalytic oxidation over Pd/carbon-zeolite and Pd/carbon-CeO nanocatalysts.

Keywords： Pd/carbon-CeO<sub>2sub>     Pd/carbon-zeolite     pine cone     ZnCl<sub>2sub>     catalytic oxidation     xylene    

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Facile synthesis and enhanced visible-light photocatalytic activity of Ti

Xiaojie Zhang,Lei Wang,Shuqing Chen,Yi Huang,Zhuonan Song,Miao Yu

Frontiers of Chemical Science and Engineering 2015, Volume 9, Issue 3,   Pages 349-358 doi: 10.1007/s11705-015-1523-5

Abstract: Ti -doped TiO nanosheets with tunable phase composition (doped TiO (A/R)) were synthesized via a hydrothermalmethod with high surface area anatase TiO nanosheets TiO (A) as a substrate, structure directing agentXRD and HRTEM measurements confirmed the existence of anatase-rutile phase junction, while Ti and single-electron-trappedsynthesis conditions, CH generation rate of doped TiO (A/R) was 2.3 times that of Ti -doped rutileTiO .

Keywords： Ti3+-doped TiO<sub>2sub>     photocatalytic CO<sub>2sub> conversion     visible light irradiation    

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All-inorganic TiO/CsAgBiBr composite as highly efficient photocatalyst under visible light irradiation

Frontiers of Chemical Science and Engineering 2023, Volume 17, Issue 12,   Pages 1925-1936 doi: 10.1007/s11705-023-2344-6

Abstract: In this work, this photocatalytic process was facilitated by a unique TiO<sub>2sub>/Cs<sub>2sub>AgBiBrTiO<sub>2sub>/Cs<sub>2sub>AgBiBr<sub>6sub> composite was investigated for its structure and photocatalyticThe results showed that when the perovskite dosage is 40%, the photocatalytic rate of TiO<sub>2sub><sub>2sub>/Cs<sub>2sub>AgBiBr<sub>6sub> composites, which will facilitate the generation of newideas for improving TiO<sub>2sub>’s photocatalytic performance.

Keywords： Cs<sub>2sub>AgBiBr<sub>6sub> nanocrystals     visible-light photocatalyst     Cs<sub>2sub>AgBiBr<sub>6sub>/TiO<sub>2sub> heterojunction    

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Effects of Pd doping on N

Mingxin Dong, Jun Wang, Jinxin Zhu, Jianqiang Wang, Wulin Wang, Meiqing Shen

Frontiers of Environmental Science & Engineering 2017, Volume 11, Issue 6, doi: 10.1007/s11783-017-0976-9

Abstract: Three types of catalysts, Pt/BaO/Al O , Pt/Pd mechanical mixing catalyst (Pt/BaO/Al O +Pd/Al O ) andPt-Pd co-impregnation catalyst (Pt-Pd/BaO/Al O ) were prepared by incipient wetness impregnation methodand reduction process, while an opposite trend was found over (Pt-Pd/BaO/Al O +Al O ).Most of N O formed over (Pt-Pd/BaO/Al O +Al O ) was originated from Pd/BaO/Al O component.H -TPR results indicated Pd-Ba interaction resulted in more difficult-to-reduce PdO species over Pd/

Keywords： NO<sub>xsub> storage reduction     Pt/BaO/Al<sub>2sub>O<sub>3sub>     Pd doping     N<sub>2sub>O formation    

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An electrochemical process that uses an Fe

Chaojie Jiang, Lifen Liu, John C. Crittenden

Frontiers of Environmental Science & Engineering 2016, Volume 10, Issue 4, doi: 10.1007/s11783-016-0860-z

Abstract: A bio-electrochemical fuel cell reactor with cathodic Fe /TiO generates electricity.It destroys recalcitrant pollutants in cathode chamber without photocatalysis.Fe /TiO generates reactive oxygenated species in the dark or under photocatalysis.electrochemical catalysis (PEC or EC) in a microbial fuel cell (MFC) was configured using a stainless-steel (SS) cathodecoated with Fe /TiO .

Keywords： Bio-anode     Photocatalytic cathode     Fe0/TiO<sub>2sub>     ESR     Dye and antibiotics     Advanced oxidation    

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Engineering a Coordinatively Unsaturated Au–O–Ti3+ Structure Toward Unprecedented H<sub>2sub> Efficiency for Low-Temperature Propene Epoxidation with H<sub>2sub> and O<sub>2sub> Article

Zhaoning Song, Hao Yan, Juncong Yuan, Hongfei Ma, Jianlin Cao, Yongxiang Wang, Qiang Wang, Chong Peng, Feng Deng, Xiang Feng, De Chen, Chaohe Yang, Yongkang Hu

Engineering 2023, Volume 25, Issue 6,   Pages 144-156 doi: 10.1016/j.eng.2023.01.008

Abstract: as the active sites for propene epoxidation with H<sub>2sub> and O<sub>2sub> at a relatively hightemperature, although they are limited by poor H<sub>2sub> efficiency.<sub>2sub> adsorption ability of the catalyst and promoting the in situ formation of H<sub>2sub>O<sub>2sub> and the Ti–OOH intermediate, even at a low temperature.The insights and methodology reported here not only shed new light on maximizing H<sub>2sub> efficiency

Keywords： Propene epoxidation     H<sub>2sub> efficiency     Au/Ti bifunctional catalysts     Coordinatively unsaturatedTi     Density-functional theory    

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Simultaneous removal of NO and chlorobenzene on VO/TiO granular catalyst: Kinetic study and performance

Frontiers of Environmental Science & Engineering 2021, Volume 15, Issue 4, doi: 10.1007/s11783-020-1363-5

Abstract:

• A V<sub>2sub>O<sub>5sub>/TiO<sub>2sub> granular catalyst for

Keywords： NO<sub>xsub>     Chlorobenzene     Simultaneous removal     Kinetic study     Performance prediction     V<sub>2sub>O<sub>5sub>/TiO<sub>2sub>     Graphical abstract    

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Promoting effect of Zr on the catalytic combustion of methane over Pd/γ-Al

Hongbo NA,Tianle ZHU,Zhiming LIU,Yifei SUN

Frontiers of Environmental Science & Engineering 2014, Volume 8, Issue 5,   Pages 659-665 doi: 10.1007/s11783-013-0613-1

Abstract: The effect of Zr on the catalytic performance of Pd/γ-Al O for the methane combustion was investigatedThe results show that the addition of Zr can improve the activity and stability of Pd/γ-Al O catalystThe active phase of methane combustion over supported palladium catalyst is the Pd /Pd mixture.Zr addition inhibits Pd aggregation and enhances the redox properties of active phase Pd / Pd .(Pd / Pd ).

Keywords： Pd-Zr/Al<sub>2sub>O<sub>3sub>     methane     catalytic combustion     catalyst regeneration    

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grown TiN/N-TiO composite for enhanced photocatalytic H evolution activity

Frontiers in Energy 2021, Volume 15, Issue 3,   Pages 721-731 doi: 10.1007/s11708-021-0766-8

Abstract: Titanium nitride (TiN) decorated N-doped titania (N-TiO<sub>2sub>) composite (TiN/N-TiO<sub>2sub>) is fabricated via an in situ nitridation using a hydrothermally synthesized TiO<sub>2sub>After the optimization of the reaction condition, the resultant TiN/N-TiO<sub>2sub> composite delivers<sub>2sub> and TiN alone, respectively.<sub>2sub> composite photocatalysts for high-efficiency water splitting.

Keywords： photocatalytic H<sub>2sub> evolution     TiN/N-TiO<sub>2sub> composite     plasmonic effect     in-situ    

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Fabrication and photocatalytic ability of an Au/TiO<sub>2sub>

Fenghe Lv, Hua Wang, Zhangliang Li, Qi Zhang, Xuan Liu, Yan Su

Frontiers of Environmental Science & Engineering 2018, Volume 12, Issue 1, doi: 10.1007/s11783-017-0977-8

Abstract: A new type of Au/TiO /reduced graphene oxide (RGO) nanocomposite was fabricated by the hydrothermal synthesisof TiO on graphene oxide followed by the photodeposition of Au nanoparticles.Au/TiO /RGO had a better photocatalytic activity than Au/TiO for the degradation of phenol.Electrochemical measurements indicated that Au/TiO /RGO had an improved charge transfer capability.Meanwhile, chemiluminescent analysis and electron spin resonance spectroscopy revealed that Au/TiO /RGO

Keywords： Reduced graphene oxide     Au     TiO<sub>2sub>     Nanocomposite     Photocatalysis    

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A study on the catalytic performance of Pd/γ-Al

Ruizhi CHU, Xianyong WEI, Zhimin ZONG, Wenjia ZHAO

Frontiers of Chemical Science and Engineering 2010, Volume 4, Issue 4,   Pages 452-456 doi: 10.1007/s11705-010-0522-9

Abstract: A series of Pd/γ-Al O hybrid catalysts were prepared by impregnation and subsequent calcination undermicrowave irradiation on the catalytic property was mainly attributed to both the higher dispersion of Pdand the significant increase in the adsorption on the CO-bridge of Pd.CO-bridge adsorption and thereby decreased the catalytic activity, whereas the coverage by metallic Pd

Keywords： Pd/γ-Al<sub>2sub>O<sub>3sub>     direct synthesis     dimethyl ether     calcination under microwave irradiation    

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g-CN-coated MnO hollow nanorod cathode for stable aqueous Zn-ion batteries

Frontiers of Chemical Science and Engineering 2023, Volume 17, Issue 2,   Pages 217-225 doi: 10.1007/s11705-022-2214-7

Abstract: Herein, superior α-MnO<sub>2sub>@g-C<sub>3sub>N<sub>4sub> was successfully prepared forstable zinc-ion batteries (ZIBs) cathode by introducing g-C<sub>3sub>N<sub>4sub> nanosheets.Compared with pure α-MnO<sub>2sub>, α-MnO<sub>2sub>@g-C<sub>3sub>N<sub>4sub> hasEven at 1 A·g–1, the α-MnO<sub>2sub>@g-C<sub>3sub>N<sub>4sub> still retains 100The α-MnO<sub>2sub>@g-C<sub>3sub>N<sub>4sub>-based cathode has the highest energy density

Keywords： α-MnO<sub>2sub> hollow nanorods     g-C<sub>3sub>N<sub>4sub>     heterojunction     aqueous Zn-ion    

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Title Author Date Type Operation

Efficient dechlorination of 2,4-dichlorophenol in an aqueous media with a mild pH using a Pd/TiO

Jiangkun DU,Jianguo BAO,Wei HU

Journal Article

Effective regeneration of thermally deactivated commercial V-W-Ti catalysts

Xuesong SHANG, Jianrong LI, Xiaowei YU, Jinsheng CHEN, Chi HE

Journal Article

Interfacial charge transfer and photocatalytic activity in a reverse designed BiO/TiO core-shell

Journal Article

Synthesis, physicochemical characterizations and catalytic performance of Pd/carbon-zeolite and Pd/carbon-CeO

Zeinab JAMALZADEH, Mohammad HAGHIGHI, Nazli ASGARI

Journal Article

Facile synthesis and enhanced visible-light photocatalytic activity of Ti

Xiaojie Zhang,Lei Wang,Shuqing Chen,Yi Huang,Zhuonan Song,Miao Yu

Journal Article

All-inorganic TiO/CsAgBiBr composite as highly efficient photocatalyst under visible light irradiation

Journal Article

Effects of Pd doping on N

Mingxin Dong, Jun Wang, Jinxin Zhu, Jianqiang Wang, Wulin Wang, Meiqing Shen

Journal Article

An electrochemical process that uses an Fe

Chaojie Jiang, Lifen Liu, John C. Crittenden

Journal Article

Engineering a Coordinatively Unsaturated Au–O–Ti3+ Structure Toward Unprecedented H<sub>2sub> Efficiency for Low-Temperature Propene Epoxidation with H<sub>2sub> and O<sub>2sub>

Zhaoning Song, Hao Yan, Juncong Yuan, Hongfei Ma, Jianlin Cao, Yongxiang Wang, Qiang Wang, Chong Peng, Feng Deng, Xiang Feng, De Chen, Chaohe Yang, Yongkang Hu

Journal Article

Simultaneous removal of NO and chlorobenzene on VO/TiO granular catalyst: Kinetic study and performance

Journal Article

Promoting effect of Zr on the catalytic combustion of methane over Pd/γ-Al

Hongbo NA,Tianle ZHU,Zhiming LIU,Yifei SUN

Journal Article

grown TiN/N-TiO composite for enhanced photocatalytic H evolution activity

Journal Article

Fabrication and photocatalytic ability of an Au/TiO<sub>2sub>

Fenghe Lv, Hua Wang, Zhangliang Li, Qi Zhang, Xuan Liu, Yan Su

Journal Article

A study on the catalytic performance of Pd/γ-Al

Ruizhi CHU, Xianyong WEI, Zhimin ZONG, Wenjia ZHAO

Journal Article

g-CN-coated MnO hollow nanorod cathode for stable aqueous Zn-ion batteries

Journal Article